Structural basis of profactor D activation: from a highly flexible zymogen to a novel self-inhibited serine protease, complement factor D

EMBO J. 1999 Feb 15;18(4):804-14. doi: 10.1093/emboj/18.4.804.

Abstract

The crystal structure of profactor D, determined at 2.1 A resolution with an Rfree and an R-factor of 25.1 and 20.4%, respectively, displays highly flexible or disordered conformation for five regions: N-22, 71-76, 143-152, 187-193 and 215-223. A comparison with the structure of its mature serine protease, complement factor D, revealed major conformational changes in the similar regions. Comparisons with the zymogen-active enzyme pairs of chymotrypsinogen, trypsinogen and prethrombin-2 showed a similar distribution of the flexible regions. However, profactor D is the most flexible of the four, and its mature enzyme displays inactive, self-inhibited active site conformation. Examination of the surface properties of the N-terminus-binding pocket indicates that Ile16 may play the initial positioning role for the N-terminus, and Leu17 probably also helps in inducing the required conformational changes. This process, perhaps shared by most chymotrypsinogen-like zymogens, is followed by a factor D-unique step, the re-orientation of an external Arg218 to an internal position for salt-bridging with Asp189, leading to the generation of the self-inhibited factor D.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Amino Acid Sequence
  • Binding Sites
  • Complement Factor D / chemistry*
  • Crystallography, X-Ray
  • Enzyme Activation
  • Enzyme Precursors / chemistry*
  • Humans
  • Models, Molecular
  • Molecular Sequence Data
  • Protein Conformation
  • Protein Precursors / chemistry*
  • Protein Processing, Post-Translational
  • Protein Structure, Secondary
  • Recombinant Proteins / chemistry
  • Sequence Homology, Amino Acid
  • Serine Endopeptidases / chemistry*

Substances

  • Enzyme Precursors
  • Protein Precursors
  • Recombinant Proteins
  • Serine Endopeptidases
  • CFD protein, human
  • Complement Factor D