Crystal structure determinations of oxidized and reduced pseudoazurins from Achromobacter cycloclastes. Concerted movement of copper site in redox forms with the rearrangement of hydrogen bond at a remote histidine

J Biol Chem. 1999 Jun 18;274(25):17845-52. doi: 10.1074/jbc.274.25.17845.

Abstract

The crystal structures of oxidized and reduced pseudoazurins from a denitrifying bacterium, Achromobacter cycloclastes IAM1013, have been determined at 1.35- and 1.6-A resolutions, respectively. The copper site in the oxidized state exhibits a distorted tetrahedral structure like those of other pseudoazurins. However, not only a small change of the copper geometry, but concerted peptide bond flips are identified. The imidazole ring of remote His6 has a hydrogen bonding distance of 2.73 A between N-delta1(His6) and O-gamma1(Thr36) in the oxidized protein. When the protein is reduced at pH 6.0, the imidazole ring rotates by 30.3 degrees and moves 1.00 A away from the position of the oxidized state. A new hydrogen bond between N-epsilon2(His6) and O-epsilon1(Glu4) is formed with a distance of 3.03 A, while the hydrogen bond between N-delta1(His6)-O-gamma1(Thr36) is maintained with an interatomic distance of 2.81 A. A concomitant peptide bond flip of main chain between Ile34 and Thr36 occurs.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alcaligenes / chemistry*
  • Azurin / analogs & derivatives*
  • Azurin / chemistry
  • Bacterial Proteins / chemistry
  • Binding Sites
  • Copper / chemistry
  • Crystallography, X-Ray
  • Hydrogen Bonding
  • Metalloproteins / chemistry
  • Models, Molecular
  • Oxidation-Reduction
  • Protein Conformation
  • Protein Structure, Secondary

Substances

  • Bacterial Proteins
  • Metalloproteins
  • pseudoazurin
  • Azurin
  • Copper

Associated data

  • PDB/1BQK
  • PDB/1BQR