Cloning, overexpression and mutagenesis of cDNA encoding dihydrolipoamide succinyltransferase component of the porcine 2-oxoglutarate dehydrogenase complex

Eur J Biochem. 2000 May;267(10):3005-16. doi: 10.1046/j.1432-1033.2000.01320.x.

Abstract

Dihydrolipoamide succinyltransferase (E2o) is the structural and catalytic core of the 2-oxoglutarate dehydrogenase (OGDH) complex. The cDNA encoding porcine E2o (PE2o) has been cloned. The PE2o cDNA spans 2547 bases encoding a presequence (68 amino-acid residues) and a mature protein (387 residues, Mr = 41 534). Recombinant porcine E2o (rPE2o) (residues 1-387), C- and N-terminal truncated PE2os, and site-directed mutant PE2os were overexpressed in Escherichia coli via the expression vector pET-11d and purified. The succinyltransferase activity of the rPE2o was about 2.2-fold higher than that of the native PE2o. Electron micrographs of the rPE2o negatively stained showed a cube-like structure very similar to that of the native PE2o. Deletion of five amino-acid residues from the C-terminus resulted in a complete loss of both enzymatic activity and formation of the cube-like structure, but the deletion of only the last two residues had no effect on either function, suggesting the important roles of the C-terminal leucine triplet (Leu383-384-385). Substitution of Ser306 with Ala, and Asp362 with Asn, Glu or Ala in the putative active site, and Leu383-384-385 with Ala or Asp abolished both functions. Substitution of His358 with Cys resulted in an 8.5-fold reduction in kcat, with little change in Km values for dihydrolipoamide and succinyl-CoA. However, self-assembly was not affected. These data indicate that Ser306, Asp362 and the Leu383-384-385 triplet are important residues in both the self-assembly and catalytic mechanism of PE2o.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acyltransferases / genetics*
  • Acyltransferases / isolation & purification
  • Acyltransferases / metabolism*
  • Amino Acid Sequence
  • Animals
  • Binding Sites
  • Cloning, Molecular
  • DNA, Complementary / metabolism
  • Electrophoresis, Polyacrylamide Gel
  • Escherichia coli / metabolism
  • Ketoglutarate Dehydrogenase Complex / chemistry
  • Ketoglutarate Dehydrogenase Complex / genetics*
  • Ketoglutarate Dehydrogenase Complex / metabolism*
  • Kinetics
  • Microscopy, Electron
  • Molecular Sequence Data
  • Mutagenesis, Site-Directed
  • Oligonucleotides / metabolism
  • Protein Binding
  • Recombinant Proteins / metabolism
  • Sequence Homology, Amino Acid
  • Swine

Substances

  • DNA, Complementary
  • Oligonucleotides
  • Recombinant Proteins
  • Ketoglutarate Dehydrogenase Complex
  • Acyltransferases
  • dihydrolipoamide succinyltransferase