Flavanone 8-dimethylallyltransferase in Sophora flavescens cell suspension cultures

Phytochemistry. 2000 Aug;54(7):649-55. doi: 10.1016/s0031-9422(00)00198-9.

Abstract

Dimethylallyl diphosphate: naringenin 8-dimethylallyltransferase (EC 2.5.1) was characterized. The enzyme was enantiospecific for (-)-(2S)-naringenin and utilized 3,3-dimethylallyl diphosphate as sole prenyl donor. It required Mg2+ (optimum concentration, 10 mM), and has an optimum pH of 9-10. The apparent Km values for 3,3-dimethylallyl diphosphate and naringenin were 120 and 36 microM, respectively. The microsomal fraction prenylated several other flavanones at the C-8 position less effectively as compared with naringenin. Interestingly, when 2'-hydroxynaringenin was used as a prenyl acceptor, the 8-lavandulyl (sophoraflavanone G) and the 6-dimethylallyl derivatives were formed, together with the 8-dimethylallyl derivative, leachianone G. These results suggest that the 2'-hydroxy group of naringenin plays an important role for the formation of a lavandulyl group.

MeSH terms

  • Alkyl and Aryl Transferases / isolation & purification*
  • Alkyl and Aryl Transferases / metabolism
  • Cells, Cultured
  • Chromatography, High Pressure Liquid
  • Fabaceae / chemistry*
  • Fabaceae / cytology
  • Microsomes / enzymology
  • Microsomes / metabolism
  • Plants, Medicinal*
  • Substrate Specificity

Substances

  • Alkyl and Aryl Transferases
  • dimethylallyl diphosphate naringenin 8-dimethylallyltransferase