Substrate specificity plays an important role in uncoupling the catalytic and scaffolding activities of rat testis DNA topoisomerase IIalpha

J Biomol Struct Dyn. 2001 Apr;18(5):749-60. doi: 10.1080/07391102.2001.10506704.

Abstract

Topoisomerase II (topo II) is a dyadic enzyme found in all eukaryotic cells. Topo II is involved in a number of cellular processes related to DNA metabolism, including DNA replication, recombination and the maintenance of genomic stability. We discovered a correlation between the development of postnatal testis and increased binding of topo IIalpha to the chromatin fraction. We used this observation to characterize DNA-binding specificity and catalytic properties of purified testis topo IIalpha. The results indicate that topo IIalpha binds a substrate containing the preferred site with greater affinity and, consequently, catalyzes the conversion of form I to form IV DNA more efficiently in contrast to substrates lacking such a site. Interestingly, topo IIalpha displayed high-affinity and cooperativity in binding to the scaffold associated region. In contrast to the preferred site, however, high-affinity binding of topo IIalpha to the scaffold-associated region failed to result in enhanced catalytic activity. Intriguingly, competition assays involving scaffold-associated region revealed an additional DNA-binding site within the dyadic topo IIalpha. These results implicate a dual role for topo IIalpha in vivo consistent with the notion that its sequestration to the chromatin might play a role in chromosome condensation and decondensation during spermatogenesis.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Antigens, Neoplasm
  • Binding Sites
  • Catalysis
  • Chromatin / metabolism*
  • DNA Topoisomerases, Type II* / metabolism*
  • DNA-Binding Proteins
  • Enzyme Inhibitors
  • Isoenzymes / antagonists & inhibitors
  • Isoenzymes / metabolism*
  • Male
  • Poly G
  • Rats
  • Substrate Specificity
  • Testis / enzymology*
  • Testis / growth & development
  • Topoisomerase II Inhibitors

Substances

  • Antigens, Neoplasm
  • Chromatin
  • DNA-Binding Proteins
  • Enzyme Inhibitors
  • Isoenzymes
  • Topoisomerase II Inhibitors
  • Poly G
  • poly(dG)
  • DNA Topoisomerases, Type II