Activation of caspases and induction of apoptosis by novel ribonucleotide reductase inhibitors amidox and didox

Exp Hematol. 2001 May;29(5):623-32. doi: 10.1016/s0301-472x(01)00624-5.

Abstract

Objective: Amidox and didox are two polyhydroxy-substituted benzohydroxamic acid derivatives that belong to a new class of ribonucleotide reductase (RR) inhibitors. RR is the rate-limiting enzyme for de novo deoxyribonucleotide synthesis, and its activity is significantly increased in tumor cells in proportion to the proliferation rate. Therefore, RR is a target for antitumor therapy.

Materials and methods: HL-60 and K562 leukemia cells were treated with increasing doses of amidox and didox. Thereafter, the mode of cytotoxic drug action was determined by Hoechst 33258/propidium iodide (HO/PI) double staining, annexin binding, DNA fragmentation, and caspase activation. This was correlated to the decrease in dNTP levels. Staining with HO/PI and binding of fluorescein isothiocyanate-conjugated annexin V to externalized phosphatidylserine were used to quantify apoptosis.

Results: Low doses of amidox or didox resulted in an increase of apoptotic HL-60 cells within 48 hours. Higher doses (50 microM amidox or 250 microM didox) led to rapid induction of apoptosis, which could be detected as early as 4 hours after treatment. After 48 hours with these concentrations, almost 100% of the HL-60 cells died by apoptosis without an increase in necrosis. K562 cells were found to be resistant to amidox but not to didox. In HL-60 cells, upstream caspase 8 is processed in response to didox, whereas caspases 8 and 9 are processed upon amidox treatment. Didox-induced apoptosis, but not amidox-induced apoptosis, can be correlated with the decrease in dNTP levels. The results suggests that amidox induces several apoptosis mechanisms in HL-60 cells. In contrast, only caspase 9 is activated by didox in K562 cells, and because amidox hardly induces apoptosis in this cell line, no caspase cleavage is observed.

Conclusions: Didox triggers distinct apoptosis pathways in HL-60 and K562 cells.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Annexin A5 / metabolism
  • Apoptosis / drug effects*
  • Caspase 8
  • Caspase 9
  • Caspase Inhibitors*
  • Caspases / drug effects*
  • DNA Fragmentation
  • Dose-Response Relationship, Drug
  • Enzyme Activation / drug effects
  • Enzyme Inhibitors / pharmacology*
  • Gelsolin / metabolism
  • HL-60 Cells / drug effects
  • HL-60 Cells / enzymology
  • Humans
  • Hydroxamic Acids / pharmacology*
  • K562 Cells / drug effects
  • K562 Cells / enzymology
  • Neoplasm Proteins / antagonists & inhibitors*
  • Oximes / pharmacology*
  • Phosphatidylserines / metabolism
  • Pilot Projects
  • Poly(ADP-ribose) Polymerases / metabolism
  • Ribonucleotide Reductases / antagonists & inhibitors*

Substances

  • Annexin A5
  • Caspase Inhibitors
  • Enzyme Inhibitors
  • Gelsolin
  • Hydroxamic Acids
  • Neoplasm Proteins
  • Oximes
  • Phosphatidylserines
  • Amidox
  • Ribonucleotide Reductases
  • Poly(ADP-ribose) Polymerases
  • CASP8 protein, human
  • CASP9 protein, human
  • Caspase 8
  • Caspase 9
  • Caspases
  • 3,4-dihydroxybenzohydroxamic acid