Two flavone C-glycosides, 5,7,4'-trihydroxy-3'-methoxyflavone-8-C-beta-D-xylopyranoside-2"-O-glucoside, 5,7-dihydroxy-3'-methoxy-4'-acetoxyflavone-8-C-beta-D- xylopyranoside-2"-O-glucoside and one known maltol beta-D-glucopyranoside were isolated for the first time from the Scleranthus uncinatus and their structures deduced by high field 1D and 2D 400 MHz NMR and (+) FAB-MS spectra.