Formation of conjugated Delta11Delta13-double bonds by Delta12-linoleic acid (1,4)-acyl-lipid-desaturase in pomegranate seeds

Eur J Biochem. 2002 Oct;269(19):4852-9. doi: 10.1046/j.1432-1033.2002.03184.x.

Abstract

For the biosynthesis of punicic acid (18:3Delta9Z,11E,13Z) a (11,14)-linoleoyl desaturase activity has been proposed. To isolate this acyl-lipid-desaturase, PCR-based cloning was used. This approach resulted in the isolation of two complete cDNAs. The first isolated full-length cDNA harbors a sequence of 1350 bp encoding a protein of 395 amino acids. The second cDNA was 1415 bp long encoding a protein of 387 amino acids. For functional identification proteins encoded by the cDNAs were expressed in Saccharomyces cerevisiae, and formation of newly formed fatty acids was analyzed by gas chromatography-free induction decay (GC-FID) and GC/MS. The expression of the heterologous enzymes resulted in the first case in a significant amount of linoleic acid and in the second case, after linoleic acid supplementation, in formation of punicic acid. The results presented here identify one cDNA coding for a classical Delta12-acyl-lipid-desaturase. The other one codes for a new type of (1,4)-acyl-lipid-desaturase that converts a cis double bond located in the Delta12-position of linoleic acid or gamma-linolenic acid, but not in alpha-linolenic acid, into a conjugated cis-trans double bond system.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Base Sequence
  • Chromatography, Gas
  • Cloning, Molecular
  • DNA, Complementary / genetics
  • DNA, Plant / genetics
  • Fatty Acid Desaturases / genetics
  • Fatty Acid Desaturases / metabolism*
  • Fatty Acids / chemistry
  • Fatty Acids / metabolism
  • Linoleic Acid / chemistry
  • Linoleic Acid / metabolism
  • Lythraceae / enzymology*
  • Lythraceae / genetics
  • Lythraceae / metabolism
  • Molecular Sequence Data
  • Phylogeny
  • Recombinant Proteins / genetics
  • Recombinant Proteins / metabolism
  • Saccharomyces cerevisiae / genetics
  • Seeds / enzymology
  • Sequence Homology, Amino Acid
  • Substrate Specificity

Substances

  • DNA, Complementary
  • DNA, Plant
  • Fatty Acids
  • Recombinant Proteins
  • Linoleic Acid
  • Fatty Acid Desaturases
  • delta-12 fatty acid desaturase

Associated data

  • GENBANK/AF437139
  • GENBANK/AF437140