In this paper, the contributions from the three major erosion sources in the catchments of Moreton Bay are quantified, specifically for the <10 microm sediment size class. The erosion sources are classified as (i) sheet erosion from cultivated land, (ii) sheet erosion from uncultivated land, and (iii) subsoil erosion from gullies and channels. The catchments were the Brisbane and Logan rivers as well as the coastal catchments. A GIS based analysis of erosion risk was used to define areas of high erosion potential in each of the erosion source types. Radionuclide concentrations of 137Cs and 226Ra were measured on the <10 microm fraction of eroding soils from these areas and then compared to concentrations on the same size fraction on deposited sediments within the rivers. A mixing model was then used to calculate the contributions from the different sources to the sediments. The contributions in the Brisbane and Logan catchments were found to be subsoil erosion (approximately 66 +/- 10%); sheet erosion from cultivated lands 33 +/- 10% and sheet erosion of uncultivated land 1 +/- 10%. Surface and subsoil erosion contributions from the coastal catchments were found to be variable.