A kinetic study of sugarcane sucrose synthase

Eur J Biochem. 2004 Oct;271(20):3971-7. doi: 10.1111/j.1432-1033.2004.04288.x.

Abstract

The kinetic data on sugarcane (Saccharum spp. hybrids) sucrose synthase (SuSy, UDP-glucose: D-fructose 2-alpha-D-glucosyltransferase, EC 2.4.1.13) are limited. We characterized kinetically a SuSy activity partially purified from sugarcane variety N19 leaf roll tissue. Primary plot analysis and product inhibition studies showed that a compulsory order ternary complex mechanism is followed, with UDP binding first and UDP-glucose dissociating last from the enzyme. Product inhibition studies showed that UDP-glucose is a competitive inhibitor with respect to UDP and a mixed inhibitor with respect to sucrose. Fructose is a mixed inhibitor with regard to both sucrose and UDP. Kinetic constants are as follows: Km values (mm, +/- SE) were, for sucrose, 35.9 +/- 2.3; for UDP, 0.00191 +/- 0.00019; for UDP-glucose, 0.234 +/- 0.025 and for fructose, 6.49 +/- 0.61. values were, for sucrose, 227 mm; for UDP, 0.086 mm; for UDP-glucose, 0.104; and for fructose, 2.23 mm. Replacing estimated kinetic parameters of SuSy in a kinetic model of sucrose accumulation with experimentally determined parameters of the partially purified isoform had significant effects on model outputs, with a 41% increase in sucrose concentration and 7.5-fold reduction in fructose the most notable. Of the metabolites included in the model, fructose concentration was most affected by changes in SuSy activity: doubling and halving of SuSy activity reduced and increased the steady-state fructose concentration by about 42 and 140%, respectively. It is concluded that different isoforms of SuSy could have significant differential effects on metabolite concentrations in vivo, therefore impacting on metabolic regulation.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Binding, Competitive
  • Enzyme Inhibitors / chemistry
  • Enzyme Inhibitors / metabolism
  • Enzyme Inhibitors / pharmacology
  • Fructose / chemistry
  • Fructose / metabolism
  • Fructose / pharmacology
  • Glucosyltransferases / antagonists & inhibitors
  • Glucosyltransferases / chemistry*
  • Glucosyltransferases / metabolism*
  • Isoenzymes
  • Kinetics
  • Models, Biological
  • Plant Leaves / enzymology
  • Saccharum / enzymology*
  • Substrate Specificity
  • Sucrose / chemistry
  • Sucrose / metabolism
  • Uridine Diphosphate / chemistry
  • Uridine Diphosphate / metabolism
  • Uridine Diphosphate Glucose / chemistry
  • Uridine Diphosphate Glucose / metabolism

Substances

  • Enzyme Inhibitors
  • Isoenzymes
  • Fructose
  • Sucrose
  • Uridine Diphosphate
  • Glucosyltransferases
  • sucrose synthase
  • Uridine Diphosphate Glucose