Probing peroxisomal beta-oxidation and the labelling of acetyl-CoA proxies with [1-(13C)]octanoate and [3-(13C)]octanoate in the perfused rat liver

Biochem J. 2005 Jul 15;389(Pt 2):397-401. doi: 10.1042/BJ20050144.

Abstract

We reported previously that a substantial fraction of the acetyl groups used to synthesize malonyl-CoA in rat heart is derived from peroxisomal beta-oxidation of long-chain and very-long-chain fatty acids. This conclusion was based on the interpretation of the 13C-labelling ratio (malonyl-CoA)/(acetyl moiety of citrate) measured in the presence of substrates that label acetyl-CoA in mitochondria only (ratio < 1.0) or in both mitochondria and peroxisomes (ratio > 1.0). The goals of the present study were to test, in rat livers perfused with [1-(13C)]octanoate or [3-(13C)]octanoate, (i) whether peroxisomal beta-oxidation contributes acetyl groups for malonyl-CoA synthesis, and (ii) the degree of labelling homogeneity of acetyl-CoA proxies (acetyl moiety of citrate, acetate, beta-hydroxybutyrate, malonyl-CoA and acetylcarnitine). Our data show that (i) octanoate undergoes two cycles of peroxisomal beta-oxidation in liver, (ii) acetyl groups formed in peroxisomes contribute to malonyl-CoA synthesis, (iii) the labelling of acetyl-CoA proxies is markedly heterogeneous, and (iv) the labelling of C1+2 of beta-hydroxybutyrate does not reflect the labelling of acetyl-CoA used in the citric acid cycle.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Acetates / metabolism
  • Acetyl Coenzyme A / metabolism*
  • Acetylcarnitine / metabolism
  • Animals
  • Caprylates / metabolism*
  • Carbon Isotopes
  • Citric Acid / metabolism
  • Isotope Labeling / methods*
  • Ketone Bodies / metabolism
  • Liver / metabolism*
  • Male
  • Malonyl Coenzyme A / metabolism
  • Mitochondria, Liver / metabolism
  • Oxidation-Reduction
  • Perfusion
  • Peroxisomes / metabolism*
  • Rats
  • Rats, Sprague-Dawley

Substances

  • Acetates
  • Caprylates
  • Carbon Isotopes
  • Ketone Bodies
  • Citric Acid
  • Malonyl Coenzyme A
  • Acetylcarnitine
  • Acetyl Coenzyme A
  • octanoic acid