Abstract
Bioassay-guided fractionation of the MeOH extract of the sponge Oceanapia sp. using the Helicobacter pylori enzyme, aspartyl semialdehyde dehydrogenase, ASD, to detect antibacterial activity, led to the isolation of a new pyridoacridine alkaloid, petrosamine B (1). Petrosamine B is a bright blue compound that is sparingly soluble in many organic solvents. The structure of 1 was determined from detailed NMR studies performed in TFA/D2O. Petrosamine B was found to be a weak inhibitor of ASD with an IC50 of 306 microM.
Publication types
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Research Support, Non-U.S. Gov't
MeSH terms
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Acridines / chemistry
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Acridines / isolation & purification*
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Acridines / pharmacology
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Aldehyde Dehydrogenase / antagonists & inhibitors*
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Alkaloids / chemistry
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Alkaloids / isolation & purification*
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Alkaloids / pharmacology
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Animals
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Australia
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Bacterial Proteins / antagonists & inhibitors*
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Enzyme Inhibitors / chemistry
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Enzyme Inhibitors / isolation & purification*
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Enzyme Inhibitors / pharmacology
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Helicobacter pylori / enzymology*
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Inhibitory Concentration 50
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Molecular Structure
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Phenanthrenes / chemistry
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Phenanthrenes / isolation & purification*
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Phenanthrenes / pharmacology
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Porifera / chemistry*
Substances
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Acridines
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Alkaloids
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Bacterial Proteins
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Enzyme Inhibitors
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Phenanthrenes
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petrosamine B
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Aldehyde Dehydrogenase
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aspartyl semialdehyde dehydrogenase, Helicobacter pylori