Adsorption characteristics of 2,4-dichlorophenoxyacetic acid (2,4-D) from aqueous solution on powdered activated carbon

J Environ Sci Health B. 2005;40(4):545-70. doi: 10.1081/PFC-200061533.

Abstract

The removal of 2,4-dichlorophenoxyacetic acid (2,4-D), one of the most commonly used phenoxy acid herbicides, from aqueous solution was studied by using acid-washed powdered activated carbon (PAC) as an adsorbent in a batch system. Adsorption equilibrium, kinetics, and thermodynamics were investigated as a function of initial pH, temperature, and initial 2,4-D concentration. Powdered activated carbon exhibited the highest 2,4-D uptake capacity of 333.3 mg g(-1) at 25 degrees C and an initial pH value of 2.0. Freundlich, Langmuir, and Redlich-Peterson isotherm models were used to express the equilibrium data of 2,4-D depending on temperature. Equilibrium data fitted very well to the Freundlich equilibrium model in the studied concentration range of 2,4-D at all the temperatures studied. Three simplified models including pseudo-first-order, pseudo-second-order, and saturation-type kinetic models were used to test the adsorption kinetics. It was shown that the adsorption of 2,4-D on PAC at 25, 35, and 45 degrees C could be best fitted by the saturation-type kinetic model with film and intraparticle diffusions being the essential rate-controlling steps. The activation energy of adsorption (EA) was determined as--1.69 kJ mole(-1). Using the thermodynamic equilibrium coefficients obtained at different temperatures, the thermodynamic constants of adsorption (deltaG degrees, deltaH degrees, and deltaS degrees) were also evaluated.

MeSH terms

  • 2,4-Dichlorophenoxyacetic Acid / chemistry*
  • 2,4-Dichlorophenoxyacetic Acid / pharmacokinetics
  • Adsorption
  • Charcoal / chemistry*
  • Charcoal / pharmacokinetics
  • Dose-Response Relationship, Drug
  • Herbicides / chemistry*
  • Herbicides / pharmacokinetics
  • Hydrogen-Ion Concentration
  • Kinetics
  • Models, Chemical*
  • Solutions
  • Temperature

Substances

  • Herbicides
  • Solutions
  • Charcoal
  • 2,4-Dichlorophenoxyacetic Acid