Detection of acoustic oscillations of single gold nanospheres by time-resolved interferometry

Phys Rev Lett. 2005 Dec 31;95(26):267406. doi: 10.1103/PhysRevLett.95.267406. Epub 2005 Dec 23.

Abstract

We measure the transient absorption of single gold particles with a common-path interferometer. The prompt electronic part of the signal provides images for diameters as small as 10 nm. Mechanical vibrations of single particles appear on a longer time scale (period of 16 ps for 50 nm diameter). They reveal the full heterogeneity of the ensemble, and the intrinsic damping of the vibration. We also observe a lower-frequency mode involving shear. Ultrafast pump-probe spectroscopy of individual particles opens new insight into mechanical properties of nanometer-sized objects.