Cloning and heterologous expression of the exo-beta-D-glucosaminidase-encoding gene (gls93) from a filamentous fungus, Trichoderma reesei PC-3-7

Appl Microbiol Biotechnol. 2006 Oct;72(4):687-95. doi: 10.1007/s00253-006-0320-y. Epub 2006 Apr 25.

Abstract

We have previously reported on purification and characterization of an exo-beta-D-glucosaminidase (Gls93) from culture filtrate of Trichoderma reesei PC-3-7 grown on N-acetyl-D-glucosamine (GlcNAc). The corresponding gene of Gls93 was cloned and characterized in this work. To our knowledge, this is the first report on cloning of the gene encoding fungal exo-beta-D-glucosaminidase. This gene has no introns and encodes a polypeptide of 892 amino acids (aa) containing a secretion signal of 28 amino acids. Comparison of the amino acid sequence to known proteins and phylogenetic analysis indicated that gls93 belongs to the glycoside hydrolase family (GHF) 2 and should be further classified into a new subgroup, exo-beta-D-glucosaminidase subgroup. The gls93 transcription was biphasic when T. reesei was grown on GlcNAc, suggesting that the expression of this gene may be regulated by a complex mechanism, in which multiple regulatory proteins are involved. Furthermore, gls93 could be expressed in Pichia pastoris (ca. 0.49-mg/ml culture). The recombinant Gls93 had the two molecular forms, ca. 105 and 100 kDa, whose difference is caused by N-glycosylation. Both of them had the same properties such as specific activity and substrate specificity and showed only the activity of exo-beta-D-glucosaminidase but not those of beta-galactosidase, beta-glucuronidase, and beta-mannosidase belonging to GHF2.

MeSH terms

  • Amino Acid Sequence
  • Chitin / chemistry
  • Chitin / metabolism
  • Cloning, Molecular
  • Gene Expression
  • Gene Expression Regulation, Fungal
  • Hexosaminidases / genetics
  • Hexosaminidases / metabolism*
  • Molecular Sequence Data
  • Phylogeny
  • Pichia / genetics
  • Trichoderma / enzymology*
  • Trichoderma / genetics*
  • Trichoderma / metabolism

Substances

  • Chitin
  • Hexosaminidases
  • exo-beta-D-glucosaminidase