A phase I pharmacokinetic study of HMN-214, a novel oral stilbene derivative with polo-like kinase-1-interacting properties, in patients with advanced solid tumors

Clin Cancer Res. 2006 Sep 1;12(17):5182-9. doi: 10.1158/1078-0432.CCR-06-0214.

Abstract

Purpose: HMN-214 is an oral prodrug of HMN-176, a stilbene derivative that interferes with the subcellular spatial location of polo-like kinase-1, a serine/threonine kinase that regulates critical mitotic events. We conducted a dose escalation study of HMN-214 in patients with advanced cancer to assess the safety profile and pharmacokinetics of HMN-214 and to establish the maximum tolerated dose.

Experimental design: Thirty-three patients were enrolled onto four dosing cohorts of HMN-214 from 3 to 9.9 mg/m2/d using a continuous 21-day dosing schedule every 28 days, with pharmacokinetic sampling during cycle 1.

Results: A severe myalgia/bone pain syndrome and hyperglycemia were dose-limiting toxicities at 9.9 mg/m2/d. A dose reduction and separate enrollment by pretreatment status (lightly versus heavily pretreated) was undertaken, with one dose-limiting toxicity (grade 3 bone pain) at 8 mg/m2/d. The maximum tolerated dose was defined as 8 mg/m2/d for both treatment cohorts. Dose-proportional increases were observed in AUC but not Cmax. There was no accumulation of HMN-176, the metabolite of HMN-214, with repeated dosing. Seven of 29 patients had stable disease as best tumor response, including 6-month stable disease in a heavily pretreated breast cancer patient. A transient decline in carcinoembryonic antigen in a patient with colorectal cancer was noted.

Conclusions: The maximum tolerated dose and recommended phase II dose of HMN-214 when administered on this schedule was 8 mg/m2/d regardless of pretreatment status. Further development of HMN-214 will focus on patient populations for which high expression of polo-like kinase-1 is seen (i.e., prostate and pancreatic cancer patients).

Publication types

  • Clinical Trial, Phase I
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Administration, Oral
  • Adult
  • Aged
  • Benzylidene Compounds / blood
  • Benzylidene Compounds / urine
  • Cell Cycle Proteins / drug effects*
  • Cohort Studies
  • Cyclic N-Oxides / administration & dosage
  • Cyclic N-Oxides / adverse effects
  • Cyclic N-Oxides / pharmacokinetics*
  • Disease Progression
  • Dose-Response Relationship, Drug
  • Drug Administration Schedule
  • Female
  • Follow-Up Studies
  • Humans
  • Male
  • Maximum Tolerated Dose
  • Middle Aged
  • Molecular Structure
  • Neoplasms / drug therapy*
  • Polo-Like Kinase 1
  • Protein Serine-Threonine Kinases / drug effects*
  • Proto-Oncogene Proteins / drug effects*
  • Pyridines / administration & dosage
  • Pyridines / adverse effects
  • Pyridines / blood
  • Pyridines / pharmacokinetics*
  • Pyridines / urine
  • Stilbenes / administration & dosage
  • Stilbenes / adverse effects
  • Stilbenes / pharmacokinetics*
  • Structure-Activity Relationship
  • Sulfonamides / administration & dosage
  • Sulfonamides / adverse effects
  • Sulfonamides / pharmacokinetics*
  • Treatment Outcome

Substances

  • (E)-4-((2-N-(4-methoxybenzenesulfonyl)amino)stilbazole)1-oxide
  • (E)-4-(2-(2-(N-acetyl-N-(4-methoxybenzenesulfonyl)amino)stilbazole)) 1-oxide
  • Benzylidene Compounds
  • Cell Cycle Proteins
  • Cyclic N-Oxides
  • Proto-Oncogene Proteins
  • Pyridines
  • Stilbenes
  • Sulfonamides
  • Protein Serine-Threonine Kinases