New insights into the alternative D-glucarate degradation pathway

J Biol Chem. 2008 Jun 6;283(23):15638-46. doi: 10.1074/jbc.M800487200. Epub 2008 Mar 25.

Abstract

Although the D-glucarate degradation pathway is well characterized in Escherichia coli, genetic and biochemical information concerning the alternative pathway proposed in Pseudomonas species and Bacillus subtilis remains incomplete. Acinetobacter baylyi ADP1 is a Gram-negative soil bacterium possessing the alternative pathway and able to grow using D-glucarate as the only carbon source. Based on the annotation of its sequenced genome (1), we have constructed a complete collection of singlegene deletion mutants (2). High throughput profiling for growth on a minimal medium containing D-glucarate as the only carbon source for approximately 2450 mutants led to the identification of the genes involved in D-glucarate degradation. Protein purification after recombinant production in E. coli allowed us to reconstitute the enzymatic pathway in vitro. We describe here the kinetic characterization of D-glucarate dehydratase, d-5-keto-4-deoxyglucarate dehydratase, and of cooperative alpha-ketoglutarate semialdehyde dehydrogenase. Transcription and expression analyses of the genes involved in D-glucarate metabolism within a single organism made it possible to access information regarding the regulation of this pathway for the first time.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acinetobacter / enzymology*
  • Acinetobacter / genetics
  • Bacterial Proteins / biosynthesis*
  • Bacterial Proteins / genetics
  • Gene Deletion
  • Gene Expression Regulation, Bacterial / physiology*
  • Gene Expression Regulation, Enzymologic / physiology*
  • Genome, Bacterial / physiology
  • Glutarates / metabolism*
  • Hydro-Lyases / biosynthesis*
  • Hydro-Lyases / genetics
  • Recombinant Proteins / biosynthesis
  • Recombinant Proteins / genetics
  • Transcription, Genetic / physiology

Substances

  • Bacterial Proteins
  • Glutarates
  • Recombinant Proteins
  • Hydro-Lyases
  • glucarate dehydratase