One-pot three-component Mannich-type reactions using sulfamic acid catalyst under ultrasound irradiation

Ultrason Sonochem. 2009 Aug;16(6):758-62. doi: 10.1016/j.ultsonch.2009.03.008. Epub 2009 Mar 27.

Abstract

Sulfamic acid (NH(2)SO(3)H, SA) was used as an efficient, inexpensive, non-toxic and recyclable green catalyst for the ultrasound-assisted one-pot Mannich reaction of aldehydes with ketones and amines. This ultrasound protocol has advantages of high yield, mild condition, no environmental pollution, and simple work-up procedures. Most importantly, beta-aminocarbonyl compounds with ortho-substituted aromatic amines are obtained in acceptable to good yields by this methodology for the first time.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Aldehydes / chemistry
  • Catalysis
  • Ethanol / chemistry
  • Mannich Bases / chemistry*
  • Solvents / chemistry
  • Sonication
  • Sulfonic Acids / chemistry*
  • Ultrasonics*

Substances

  • Aldehydes
  • Mannich Bases
  • Solvents
  • Sulfonic Acids
  • Ethanol
  • sulfamic acid