Abstract
The filipin biosynthetic gene cluster of Streptomyces avermitilis contains pteB, a homolog of crotonyl-CoA carboxylase/reductase. PteB was predicted to be 2-octenoyl-CoA carboxylase/reductase, supplying hexylmalonyl-CoA to filipin biosynthesis. Recombinant PteB displayed selective reductase activity toward 2-octenoyl-CoA while generating a broad range of alkylmalonyl-CoAs in the presence of bicarbonate.
Publication types
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Research Support, Non-U.S. Gov't
MeSH terms
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Acyl Coenzyme A / metabolism*
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Acyl-CoA Dehydrogenases / chemistry
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Acyl-CoA Dehydrogenases / genetics
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Acyl-CoA Dehydrogenases / metabolism*
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Anti-Bacterial Agents / chemistry*
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Chromatography, High Pressure Liquid
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Cloning, Molecular
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Electrophoresis, Polyacrylamide Gel
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Escherichia coli
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Filipin* / biosynthesis
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Multigene Family
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Plasmids
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Sequence Homology, Amino Acid
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Spectrophotometry
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Streptomyces / chemistry
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Streptomyces / enzymology*
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Streptomyces / genetics
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Transformation, Bacterial
Substances
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Acyl Coenzyme A
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Anti-Bacterial Agents
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octenoyl-coenzyme A
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Filipin
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crotonyl-coenzyme A
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Acyl-CoA Dehydrogenases
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acyl-CoA dehydrogenase (NADP+)