Pathway for lipid A biosynthesis in Arabidopsis thaliana resembling that of Escherichia coli

Proc Natl Acad Sci U S A. 2011 Jul 12;108(28):11387-92. doi: 10.1073/pnas.1108840108. Epub 2011 Jun 27.

Abstract

The lipid A moiety of Escherichia coli lipopolysaccharide is a hexa-acylated disaccharide of glucosamine that makes up the outer monolayer of the outer membrane. Arabidopsis thaliana contains nuclear genes encoding orthologs of key enzymes of bacterial lipid A biosynthesis, including LpxA, LpxC, LpxD, LpxB, LpxK and KdtA. Although structurally related lipid A molecules are found in most other gram-negative bacteria, lipid A and its precursors have not been directly detected in plants previously. However, homozygous insertional knockout mutations or RNAi knock-down constructs of Arabidopsis lpx and kdtA mutants revealed accumulation (or disappearance) of the expected monosaccharide or disaccharide lipid A precursors by mass spectrometry of total lipids extracted from 10-day old seedlings of these mutants. In addition, fluorescence microscopy of lpx-gfp fusions in transgenic Arabidopsis plants suggests that the Lpx and KdtA proteins are expressed and targeted to mitochondria. Although the structure of the lipid A end product generated by plants is still unknown, our work demonstrates that plants synthesize lipid A precursors using the same enzymatic pathway present in E. coli.

Publication types

  • Comparative Study
  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acyltransferases / genetics
  • Acyltransferases / metabolism
  • Arabidopsis / genetics
  • Arabidopsis / metabolism*
  • Base Sequence
  • Chromosome Mapping
  • DNA, Plant / genetics
  • Escherichia coli / genetics
  • Escherichia coli / metabolism*
  • Gene Knockdown Techniques
  • Gene Knockout Techniques
  • Genes, Plant
  • Glycolipids / metabolism
  • Lipid A / biosynthesis*
  • Lipid A / chemistry
  • Lipid A / genetics
  • Metabolic Networks and Pathways
  • Mitochondria / metabolism
  • Molecular Structure
  • Mutation
  • Plants, Genetically Modified
  • Species Specificity

Substances

  • DNA, Plant
  • Glycolipids
  • Lipid A
  • lipid X
  • Acyltransferases