Metabolism profile of timosaponin B-II in urine after oral administration to rats by ultrahigh-performance liquid chromatography/quadrupole-time-of-flight mass spectrometry

Rapid Commun Mass Spectrom. 2012 Sep 15;26(17):1955-64. doi: 10.1002/rcm.6299.

Abstract

Rationale: Timosaponin B-II (TB-II) is one of the major bioactive steroid glycosides isolated from Anemarrhena asphodeloides Bge. (Fam. Liliaceae). It has been regarded as a potential lead compound, which may be further developed into a promising new drug for preventing dementia. To fully understand the action mechanism of TB-II, it is important to study the metabolism profile of this compound in vivo.

Methods: Herein, a rapid and sensitive method based on ultrahigh-performance liquid chromatography (UHPLC)/quadrupole-time-of-flight mass spectrometry (QTOFMS) was established to comprehensively investigate the metabolism of TB-II in Sprague-Dawley rat urine following oral administration of a single dose of TB-II at 500.4 mg·kg(-1).

Results: A total of twelve metabolites were detected and identified by means of comparing molecular mass, retention time and spectral pattern of the analytes with those of the parent drug. A possible metabolic pathway on the biotransformation of TB-II was also investigated and proposed.

Conclusions: Oxidation, deglycosylation and E-ring cleavage were found to be the major metabolic processes of the compound in rat. It is the first report on a mammalian metabolism study of timosaponin, a common member of steroid glycosides, in rat urine.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Administration, Oral
  • Animals
  • Biotransformation
  • Chromatography, High Pressure Liquid / methods*
  • Male
  • Mass Spectrometry / methods*
  • Metabolic Networks and Pathways
  • Rats
  • Rats, Sprague-Dawley
  • Saponins / administration & dosage
  • Saponins / chemistry
  • Saponins / pharmacokinetics*
  • Saponins / urine*
  • Sensitivity and Specificity
  • Steroids / administration & dosage
  • Steroids / chemistry
  • Steroids / pharmacokinetics*
  • Steroids / urine*

Substances

  • Saponins
  • Steroids
  • timosaponin B-II