Terahertz excitation of a coherent λ-type three-level system of exciton-polariton modes in a quantum-well microcavity

Phys Rev Lett. 2012 Jun 29;108(26):267402. doi: 10.1103/PhysRevLett.108.267402. Epub 2012 Jun 26.

Abstract

Interactions of few-cycle terahertz pulses with the induced optical polarization in a quantum-well microcavity reveal that the lower and higher exciton-polariton modes together with the optically forbidden 2p-exciton state form a unique Λ-type three-level system. Pronounced nonlinearities are observed via time-resolved strong-terahertz and weak-optical excitation spectroscopy and explained with a fully microscopic theory. The results show that the terahertz pulses strongly couple the exciton-polariton states to the 2p-exciton state while no resonant transition between the two polariton levels is observed.