Density-driven convection enhanced by an inclined boundary: implications for geological CO2 storage

Phys Rev E Stat Nonlin Soft Matter Phys. 2013 Jan;87(1):011003. doi: 10.1103/PhysRevE.87.011003. Epub 2013 Jan 31.

Abstract

We experimentally examine dissolution-generated, density-driven convection with an inclined boundary in both a Hele-Shaw cell and in a porous medium. The convection, manifested by descending, dense fingers, is generated by a diffusive mixing of two liquids at the interface. We investigate the dynamics, widths, and wavelengths of the fingers and characterize the global convective transport for a wide range of permeabilities and tilt angles of the boundaries. Our results have implications for CO(2) storage in a saline aquifer when brine saturated with CO(2) produces a heavier mixture, which may result in an enhanced mass transfer by convection. Our measurements reveal a further enhancement of convection with inclined boundaries, which suggests that sloping formations provide improved sites for CO(2) storage.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Carbon Dioxide / chemistry*
  • Carbon Dioxide / isolation & purification*
  • Computer Simulation
  • Diffusion
  • Groundwater / chemistry*
  • Models, Chemical*
  • Models, Molecular*

Substances

  • Carbon Dioxide