Washing effects of limonene on pesticide residues in green peppers

J Sci Food Agric. 2013 Sep;93(12):2917-21. doi: 10.1002/jsfa.6080. Epub 2013 Mar 13.

Abstract

Background: The presence of pesticide residues in food has caused much concern. The low health risks and environmental impacts of limonene make it a very interesting solvent for use in green chemistry. Washing effects of limonene on pesticide residues of methyl chlorpyrifos, chlorothalonil, chlorpyrifos, fenpropathrin and deltamethrin were investigated in green pepper.

Results: Results showed that washing with a low concentration of limonene for 5 min (where LOQ is limit of quantitation) caused 53.67%, <LOQ, 64.29%, 68.69% and 66.22% loss of the above pesticides, respectively, while corresponding values of washing with a high concentration were 84.64%, <LOQ, 90.46%, 89.00% and 89.36%, respectively. Washing with a low concentration of limonene for 10 min produced 55.90%, <LOQ, 66.19%, 72.08% and 73.25% loss, respectively, while corresponding values of washing with a high concentration were 94.42%, <LOQ, 96.58%, 92.04% and < LOQ, respectively. The reductions due to washing with tap water (for 10 min) and the emulsion with only egg yolk lecithin (at high concentration for 10 min) were 25.18 %, 37.83%, 21.84%, 20.87%, 13.86% and < LOQ, 59.70%, 54.09%, 54.76%, 54.47%, respectively.

Conclusion: The data indicated that washing with a low concentration of limonene for 5 min was the optimal treatment for elimination of pesticide residues in green pepper, considering effect and treatment time as well as cost.

Keywords: green pepper; green washing detergent; limonene; pesticide residues.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Capsicum / chemistry*
  • China
  • Chlorpyrifos / analogs & derivatives
  • Chlorpyrifos / analysis
  • Chromatography, Gas
  • Cyclohexenes / chemistry*
  • Detergents / chemistry*
  • Emulsions
  • Food Contamination / prevention & control*
  • Food Handling*
  • Fruit / chemistry*
  • Fungicides, Industrial / analysis
  • Insecticides / analysis
  • Limit of Detection
  • Limonene
  • Nitriles / analysis
  • Osmolar Concentration
  • Pesticide Residues / analysis*
  • Pesticide Residues / chemistry
  • Pyrethrins / analysis
  • Solvents / chemistry
  • Terpenes / chemistry*
  • Time Factors

Substances

  • Cyclohexenes
  • Detergents
  • Emulsions
  • Fungicides, Industrial
  • Insecticides
  • Nitriles
  • Pesticide Residues
  • Pyrethrins
  • Solvents
  • Terpenes
  • decamethrin
  • fenpropathrin
  • Limonene
  • tetrachloroisophthalonitrile
  • Chlorpyrifos
  • chlorpyrifos-methyl