[2+2+2] cyclotrimerization of alkynes and isocyanates/isothiocyanates catalyzed by ruthenium-alkylidene complexes

J Org Chem. 2013 Oct 4;78(19):9995-10001. doi: 10.1021/jo401538p. Epub 2013 Sep 12.

Abstract

Ruthenium carbene catalysts are able to catalyze crossed [2+2+2] cyclotrimerizations of α,ω-diynes with isocyanates, isothiocyanates, and carbon disulfide. Both aliphatic and aromatic isocyanates can be used to produce fused 2-pyridones, although aliphatic isocyanates were more reactive. Aromatic isocyanates give better results when they bear electron-donating substituents. The reaction of unsymmetrical α,ω-diynes gave a product only with the substituent adjacent to the 2-pyridone nitrogen. Isothiocyanates gave thiopyranimines upon reaction with the C═S bond, whereas CS2 reacted efficiently to give a thioxothiopyrane.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alkynes / chemistry*
  • Catalysis
  • Coordination Complexes / chemistry*
  • Cyclization
  • Cycloparaffins / chemistry*
  • Isocyanates / chemistry*
  • Isothiocyanates / chemistry*
  • Ruthenium
  • Stereoisomerism

Substances

  • Alkynes
  • Coordination Complexes
  • Cycloparaffins
  • Isocyanates
  • Isothiocyanates
  • isothiocyanic acid
  • Ruthenium