Determination of ammonia by designing an optode based on immobilization of a Co(III)-Schiff base complex on a triacetylcelluose membrane

J AOAC Int. 2014 Jan-Feb;97(1):259-62. doi: 10.5740/jaoacint.11-430.

Abstract

A novel ammonia optode was designed using [4-methyl-N,N'-bis(salicylidene)-1,2-phenylenediamine] tributylphosphincobalt(III) perchlorate monohydrate [Co(4-MeSaloph)(PBu)3]+ complex coated on a triacetylcellulose membrane. The sensor could be used at a wavelength of 378 nm to detect ammonia in the range of 8.3 x 10(-4) and -1.25 x 10(-2) M in borate buffer (pH 10). The LOD was found to be 9.5 x 10(-5) M. The response time of the optode was 2-3 min and depended on the concentration of ammonia. This optode was successfully applied for the determination of ammonia in drinking water.

MeSH terms

  • Ammonia / chemistry*
  • Cellulose / analogs & derivatives*
  • Cellulose / chemistry
  • Cobalt / chemistry*
  • Hydrogen-Ion Concentration
  • Membranes, Artificial*
  • Optical Devices*
  • Schiff Bases / chemistry*

Substances

  • Membranes, Artificial
  • Schiff Bases
  • Cobalt
  • Ammonia
  • Cellulose
  • cellulose triacetate