Bioassay-guided isolation and identification of anti-platelet-active compounds from the root of Ashitaba (Angelica keiskei Koidz.)

Nat Prod Res. 2014;28(24):2312-6. doi: 10.1080/14786419.2014.931389. Epub 2014 Jul 14.

Abstract

Platelet aggregation is fundamental to a wide range of physiological and pathological processes, including the induction of thrombosis and arteriosclerosis. Anti-platelet activity of a crude methanol extract and solvent fractions of Ashitaba roots (Angelica keiskei Koidz.) was evaluated using a turbidimetric method using washed rabbit platelets. We identified the anti-platelet activities of two chalcones, 4-hydroxyderricin and xanthoangelol, isolated from the ethyl acetate-soluble fraction of Ashitaba roots by using a bioassay-guided isolation method. 4-Hydroxyderricin and xanthoangelol effectively inhibited platelet aggregation induced by collagen (IC50 of 41.9 and 35.9 μM, respectively), platelet-activating factor (IC50 of 46.1 and 42.3 μM, respectively) and phorbol 12-myristate 13-acetate (IC50 of 16.5 and 45.9 μM, respectively). These compounds did not inhibit thrombin-induced platelet aggregation (IC50 of>80 μM). The results suggest that the chalcones 4-hydroxyderricin and xanthoangelol may be potent anti-thrombotic components of A. keiskei Koidz.

Keywords: 4-hydroxyderricin; Angelica keiskei Koidaz; Ashitaba; anti-platelet; xanthoangelol.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Angelica / chemistry*
  • Animals
  • Antifibrinolytic Agents / chemistry
  • Antifibrinolytic Agents / isolation & purification*
  • Antifibrinolytic Agents / pharmacology*
  • Biological Assay
  • Chalcone / analogs & derivatives*
  • Chalcone / chemistry
  • Chalcone / isolation & purification
  • Chalcone / pharmacology
  • Inhibitory Concentration 50
  • Plant Roots / chemistry
  • Platelet Aggregation Inhibitors / chemistry
  • Platelet Aggregation Inhibitors / isolation & purification*
  • Platelet Aggregation Inhibitors / pharmacology*
  • Rabbits

Substances

  • Antifibrinolytic Agents
  • Platelet Aggregation Inhibitors
  • 4-hydroxyderricin
  • Chalcone
  • xanthoangelol