Fractal Lévy Heat Transport in Nanoparticle Embedded Semiconductor Alloys

Nano Lett. 2015 Jul 8;15(7):4269-73. doi: 10.1021/nl5044665. Epub 2015 Feb 9.

Abstract

Materials with embedded nanoparticles are of considerable interest for thermoelectric applications. Here, we experimentally characterize the effect of nanoparticles on the recently discovered Lévy phonon transport in semiconductor alloys. The fractal space dimension α ≈ 1.55 of quasiballistic (superdiffusive) heat conduction in (ErAs)x:InGaAlAs is virtually independent of the Er content 0.001 < x < 0.1 but instead controlled by alloy scattering of the host matrix. The increased nanoparticle concentration does reduce the diffusive recovery length by an order of magnitude. The bulk conductivity drops by 3-fold, in close agreement with a Callaway model. Our results may provide helpful hints toward engineering superdiffusive heat transport similar to what has been achieved with light in Lévy glasses.

Keywords: Ballistic heat transport; Lévy flight; Nanoparticles; Superdiffusion; Thermal Conductivity; Thermoelectric materials.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.