Method for time-resolved monitoring of a solid state biological film using photothermal infrared nanoscopy on the example of poly-L-lysine

Anal Chem. 2015 Apr 21;87(8):4415-20. doi: 10.1021/acs.analchem.5b00241. Epub 2015 Apr 8.

Abstract

We report time-resolved photothermal infrared nanoscopy measurements across a spectral range of more than 100 cm(-1) (1565 cm(-1) to 1729 cm(-1)) at nanoscale spatial resolution. This is achieved through a custom-built system using broadly tunable external cavity quantum cascade lasers in combination with a commercially available atomic force microscope. The new system is applied to the analysis of conformational changes of a polypeptide (poly-l-lysine) film upon temperature-induced changes of the humidity in the film. Changes of the secondary structure from β-sheet to α-helix could be monitored at a time resolution of 15 s per spectrum. The time-resolved spectra are well comparable to reference measurements acquired with conventional Fourier transform infrared microscopy.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Humidity
  • Nanotechnology*
  • Photochemical Processes
  • Polylysine / analysis*
  • Spectrophotometry, Infrared
  • Temperature*
  • Time Factors

Substances

  • Polylysine