Probing and controlling liquid crystal helical nanofilaments

Nano Lett. 2015 May 13;15(5):3420-4. doi: 10.1021/acs.nanolett.5b00760. Epub 2015 Apr 21.

Abstract

We report the first in situ measurement of the helical pitch of the helical nanofilament B4 phase of bent-core liquid crystals using linearly polarized, resonant soft X-ray scattering at the carbon K-edge. A strong, anisotropic scattering peak corresponding to the half-pitch of the twisted smectic layer structure was observed. The equilibrium helical half-pitch of NOBOW is found to be 120 nm, essentially independent of temperature. However, the helical pitch can be tuned by mixing guest organic molecules with the bent-core host, followed by thermal annealing.

Keywords: B4; bent-core; carbon edge; helical pitch; helix; nanofilament; resonant soft X-ray scattering; smectic liquid crystal.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.