Elusive Sulfurous Acid: Gas-Phase Basicity and IR Signature of the Protonated Species

J Phys Chem Lett. 2015 May 7;6(9):1605-10. doi: 10.1021/acs.jpclett.5b00450. Epub 2015 Apr 15.

Abstract

The ion corresponding to protonated sulfurous acid, H3SO3(+), has been successfully delivered into the gas phase by electrospray ionization of the solution of a suitable precursor and an in-source fragmentation process. The neutral acid is a highly elusive molecule. However, its gas-phase basicity has been ascertained by means of a kinetic study of proton-transfer reactivity. The structure of the H3SO3(+) sampled ion has been probed by IRMPD spectroscopy in two complementary IR frequency ranges in conjunction with density functional theory calculations and found to conform to a trihydroxosulfonium ion. The characteristic IR signatures may aid in deciphering the presence of this species in extraterrestrial atmospheres.

Keywords: IRMPD spectroscopy; density functional theory calculations; gas-phase ion chemistry; inorganic cations; mass spectrometry; molecular structure; planet atmosphere.