[DNA polymerase I, Klenow fragment of Escherichia coli: hydrolysis and pyrophosphorolysis of DNA containing phosphothioate groups]

Mol Biol (Mosk). 1989 Mar-Apr;23(2):449-62.
[Article in Russian]

Abstract

Reaction of DNA synthesis catalyzed by DNA polymerase I KF in the presence of 2'-deoxynucleoside 5'-alpha-thiotriphosphates (dNTP alpha S) was investigated. DNA with thiophosphate groups (DNA[P=S]) obtained by such a way was studied in reactions of hydrolysis and pyrophosphorolysis catalyzed by DNA polymerase I KF. It is shown that the rate of DNA elongation is decreased both on the step of incorporation of dNMP alpha S residues and on the step of incorporation of the next dNMP residue. The rate of pyrophosphorolysis of 3'-terminal dNMP alpha S was demonstrated to be one order of magnitude less in comparison with the corresponding reaction with the natural dNMP residue. Contrary, the rate of 3'----5'-exonuclease hydrolysis of both DNA[P=S] and DNA of the same structure revealed no distinguishable differences.

MeSH terms

  • Bacteriophages / genetics
  • Base Sequence
  • Chromatography
  • DNA Polymerase I / metabolism*
  • DNA, Viral / metabolism*
  • DNA-Directed DNA Polymerase / metabolism*
  • Electrophoresis, Polyacrylamide Gel
  • Escherichia coli / enzymology*
  • Hydrolysis
  • Molecular Sequence Data
  • Organothiophosphorus Compounds / metabolism
  • Phosphorylation

Substances

  • DNA, Viral
  • Organothiophosphorus Compounds
  • DNA Polymerase I
  • DNA-Directed DNA Polymerase