Hydrogen from Water over Openly-Structured Graphitic Carbon Nitride Polymer through Photocatalysis

ChemSusChem. 2016 Mar 8;9(5):478-84. doi: 10.1002/cssc.201501520. Epub 2016 Feb 2.

Abstract

Openly-structured g-C3 N4 microspheres (CNMS) are developed through a well-controlled strategy. These materials have unique features of open 3 D structure, ordered hierarchical porosity, and improved optical and electronic properties. Hydrogen evolution from water is performed under a 300 W Xe lamp with a cut-off filter (λ>420 nm) and Pt nanoparticles are used as the co-catalyst (3.0 wt%). The catalyst prepared at 600 °C (CNMS-600) has a hydrogen evolution rate (HER) of 392 μmol h(-1) (apparent quantum yield, AQY=6.3%) at 420 nm. This value is higher than that of g-C3 N4 nanosheets prepared through thermal oxidation, liquid exfoliation, or chemical exfoliation. The HER value is only 27 μmol h(-1) (AQY=0.43%) at 420 nm for bulk g-C3 N4 from melamine. The evolution of openly-structured CNMS was investigated by TEM, FTIR, and XRD. The improved optical and electronic properties were demonstrated through UV/Vis absorption spectra, valence-band X-ray photoelectron spectroscopy, photoluminescence spectroscopy, electron paramagnetic resonance spectroscopy, and electrochemical impedance spectroscopy.

Keywords: hydrogen; nanostructures; nitrides; photocatalysis; water splitting.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Catalysis
  • Graphite / chemistry*
  • Hydrogen / chemistry*
  • Microscopy, Atomic Force
  • Microscopy, Electron, Scanning
  • Nitriles / chemistry*
  • Photochemical Processes
  • Photoelectron Spectroscopy
  • Polymers / chemistry*
  • Spectrophotometry, Ultraviolet
  • Water / chemistry*

Substances

  • Nitriles
  • Polymers
  • Water
  • cyanogen
  • Graphite
  • Hydrogen