Protective effects of marein on high glucose-induced glucose metabolic disorder in HepG2 cells

Phytomedicine. 2016 Aug 15;23(9):891-900. doi: 10.1016/j.phymed.2016.05.004. Epub 2016 May 19.

Abstract

Background: Our previous study has shown that Coreopsis tinctoria increases insulin sensitivity and regulates hepatic metabolism in high-fat diet (HFD)-induced insulin resistance rats. However, it is unclear whether or not marein, a major compound of C. tinctoria, could improve insulin resistance. Here we investigate the effect and mechanism of action of marein on improving insulin resistance in HepG2 cells.

Methods: We investigated the protective effects of marein in high glucose-induced human liver carcinoma cell HepG2. In kinase inhibitor studies, genistein, LY294002, STO-609 and compound C were added to HepG2 cells 1h before the addition of marein. Transfection with siRNA was used to knock down LKB1, and 2-(N-(7-nitrobenz-2-oxa-1, 3-diazol-4-yl) amino)-2-deoxyglucose (2-NBDG), an effective tracer, was used to detect glucose uptake.

Results: The results showed for the first time that marein significantly stimulates the phosphorylation of AMP-activated protein kinase (AMPK) and the Akt substrate of 160kDa (AS160) and enhanced the translocation of glucose transporter 1 (GLUT1) to the plasma membrane. Further study indicated that genistein (an insulin receptor tyrosine kinase inhibitor) altered the effect of marein on glucose uptake, and both LY294002 (a phosphatidylinositol 3-kinase inhibitor) and compound C (an AMP-activated protein kinase inhibitor) significantly decreased marein-stimulated 2-NBDG uptake. Additionally, marein-stimulated glucose uptake was blocked in the presence of STO-609, a CaMKK inhibitor; however, marein-stimulated AMPK phosphorylation was not blocked by LKB1 siRNA in HepG2 cells. Marein also inhibited the phosphorylation of insulin receptor substrate (IRS-1) at Ser 612, but inhibited GSK-3β phosphorylation and increased glycogen synthesis. Moreover, marein significantly decreased the expression levels of FoxO1, G6Pase and PEPCK.

Conclusions: Consequently, marein improved insulin resistance induced by high glucose in HepG2 cells through CaMKK/AMPK/GLUT1 to promote glucose uptake, through IRS/Akt/GSK-3β to increase glycogen synthesis, and through Akt/FoxO1 to decrease gluconeogenesis. Marein could be a promising leading compound for the development of hypoglycemic agent or developed as an adjuvant drug for diabetes mellitus.

Keywords: Akt; FoxO1; Gluconeogenesis; Glycogen synthesis; HepG2 cells; Marein.

MeSH terms

  • AMP-Activated Protein Kinase Kinases
  • Animals
  • Cell Line, Tumor
  • Chalcones / pharmacology*
  • Gene Knockdown Techniques
  • Gluconeogenesis / drug effects
  • Glucose / metabolism
  • Glucose / toxicity*
  • Glucose Metabolism Disorders / chemically induced*
  • Glucose Metabolism Disorders / prevention & control*
  • Glucose Transporter Type 1 / metabolism
  • Hep G2 Cells
  • Humans
  • Insulin Resistance
  • Phosphorylation / drug effects
  • Protective Agents / pharmacology*
  • Protein Kinase Inhibitors / pharmacology
  • Protein Serine-Threonine Kinases / genetics
  • RNA, Small Interfering / genetics
  • Rats

Substances

  • Chalcones
  • Glucose Transporter Type 1
  • Protective Agents
  • Protein Kinase Inhibitors
  • RNA, Small Interfering
  • SLC2A1 protein, human
  • marein
  • Protein Serine-Threonine Kinases
  • STK11 protein, human
  • AMP-Activated Protein Kinase Kinases
  • Glucose