Nanostructured ZnO-TiO2 thin film oxide as anode material in electrooxidation of organic pollutants. Application to the removal of dye Amido black 10B from water

Environ Sci Pollut Res Int. 2017 Jan;24(2):1442-1449. doi: 10.1007/s11356-016-7920-6. Epub 2016 Oct 25.

Abstract

Electrochemical oxidative degradation of diazo dye Amido black 10B (AB10B) as model pollutant in water has been studied using nanostructured ZnO-TiO2 thin films deposited on graphite felt (GrF) substrate as anode. The influence of various operating parameters, namely the current intensity, the nature and concentration of catalyst, the nature of electrode materials (anode/cathode), and the adsorption of dye and ambient light were investigated. It was found that the oxidative degradation of AB10B followed pseudo first-order kinetics. The optimal operating conditions for the degradation of 0.12 mM (74 mg L-1) dye concentration and mineralization of its aqueous solution were determined as GrF-ZnO-TiO2 thin film anode, 100 mA current intensity, and 0.1 mM Fe2+ (catalyst) concentration. Under these operating conditions, discoloration of AB10B solution was reached at 60 min while 6 h treatment needed for a mineralization degree of 91 %. Therefore, this study confirmed that the electrochemical process is effective for the degradation of AB10B in water using nanostructured ZnO-TiO2 thin film anodes.

Keywords: Amido black 10B; Electro-Fenton; Electrooxidation; Mineralization; Nanostructured ZnO-TiO2; Rate constant.

MeSH terms

  • Adsorption
  • Amido Black / isolation & purification*
  • Azo Compounds / chemistry
  • Catalysis
  • Electrodes*
  • Graphite / chemistry
  • Kinetics
  • Naphthalenesulfonates / chemistry
  • Oxidation-Reduction
  • Titanium / chemistry*
  • Water Pollutants, Chemical / isolation & purification*
  • Water Purification / methods*
  • Zinc Oxide / chemistry*

Substances

  • Azo Compounds
  • Naphthalenesulfonates
  • Naphthol Blue Black
  • Water Pollutants, Chemical
  • titanium dioxide
  • Graphite
  • Titanium
  • Zinc Oxide
  • Amido Black