Morphological Control of Heteroleptic cis- and trans-Pd2 L2 L'2 Cages

Angew Chem Int Ed Engl. 2017 Jul 3;56(28):8285-8289. doi: 10.1002/anie.201702573. Epub 2017 May 23.

Abstract

Control over the integrative self-sorting of metallo-supramolecular assemblies opens up possibilities for introducing increased complexity and function into a single self-assembled architecture. Herein, the relationship between the geometry of three ligand components and morphology of three self-sorted heteroleptic [Pd2 L2 L'2 ]4+ cages is examined. Pd-mediated assembly of two bis-monodentate pyridyl ligands with native bite angles of 75° and 120° affords a cis-[Pd2 L2 L'2 ]4+ cage while the same reaction with two ligands with bite angles of 75° and 60° gives an unprecedented, self-penetrating structural motif; a trans-[Pd2 (anti-L)2 L'2 ]4+ heteroleptic cage with a "doubly bridged figure eight" topology. Each heteroleptic assembly can be formed by cage-to-cage conversion of the homoleptic precursors and morphological control of [Pd2 L2 L'2 ] cages is achieved by selective ligand displacement transformations in a system of three ligands and at least six possible cage products.

Keywords: cage compounds; morphological control; self-sorting; supramolecular chemistry; topology.

Publication types

  • Research Support, Non-U.S. Gov't