4β-Hydroxycholesterol level significantly correlates with steady-state serum concentration of the CYP3A4 substrate quetiapine in psychiatric patients

Br J Clin Pharmacol. 2017 Nov;83(11):2398-2405. doi: 10.1111/bcp.13341. Epub 2017 Jul 21.

Abstract

Aim: 4β-Hydroxycholesterol (4βOHC) is sensitive towards induction or inhibition of CYP3A4, but its potential usefulness as a dosing biomarker remains to be demonstrated. The aim of this study was to investigate the correlation between 4βOHC levels and steady-state concentrations (Css) of quetiapine, a CYP3A4 substrate with high presystemic metabolism, in psychiatric patients.

Methods: Serum samples from 151 patients treated with quetiapine as immediate release (IR; n = 98) or slow release (XR; n = 53) tablets were included for analysis of 4βOHC. In all patients, Css of quetiapine had been measured at trough level, i.e. 10-14 and 17-25 h post-dosing for IR and XR tablets, respectively. Correlations between 4βOHC levels and dose-adjusted Css (C/D ratios) of quetiapine were tested by univariate (Spearman's) and multivariate (multiple linear regression) analyses. Gender, age (≥60 vs. <60 years) and tablet formulation were included as potential covariates in the multivariate analysis.

Results: Correlations between 4βOHC levels and quetiapine C/D ratios were highly significant both for IR- and XR-treated patients (P < 0.0001). Estimated Spearman r values were -0.47 (95% confidence interval -0.62, -0.30) and -0.56 (-0.72, -0.33), respectively. The relationship between 4βOHC level and quetiapine C/D ratio was also significant in the multiple linear regression analysis (P < 0.001), including gender (P = 0.023) and age (P = 0.003) as significant covariates.

Conclusions: The present study shows that 4βOHC level is significantly correlated with steady-state concentration of quetiapine. This supports the potential usefulness of 4βOHC as a phenotype biomarker for individualized dosing of quetiapine and other drugs where systemic exposure is mainly determined by CYP3A4 metabolism.

Keywords: 4β-hydroxycholesterol; CYP3A4; biomarker; quetiapine.

MeSH terms

  • Adolescent
  • Adult
  • Age Factors
  • Aged
  • Aged, 80 and over
  • Antipsychotic Agents / pharmacokinetics*
  • Antipsychotic Agents / therapeutic use
  • Biomarkers, Pharmacological / blood*
  • Cytochrome P-450 CYP3A / metabolism*
  • Delayed-Action Preparations / pharmacokinetics
  • Delayed-Action Preparations / therapeutic use
  • Female
  • Humans
  • Hydroxycholesterols / blood*
  • Male
  • Mental Disorders / blood
  • Mental Disorders / drug therapy*
  • Middle Aged
  • Prospective Studies
  • Quetiapine Fumarate / pharmacokinetics*
  • Quetiapine Fumarate / therapeutic use
  • Sex Factors
  • Tablets
  • Young Adult

Substances

  • Antipsychotic Agents
  • Biomarkers, Pharmacological
  • Delayed-Action Preparations
  • Hydroxycholesterols
  • Tablets
  • cholest-5-ene-3,4-diol
  • Quetiapine Fumarate
  • Cytochrome P-450 CYP3A
  • CYP3A4 protein, human