Polymer-Supported Stereoselective Synthesis of Benzoxazino[4,3-b][1,2,5]thiadiazepinone 6,6-dioxides

ACS Comb Sci. 2017 Oct 9;19(10):670-674. doi: 10.1021/acscombsci.7b00115. Epub 2017 Aug 31.

Abstract

Herein, we report the stereoselective synthesis of trisubstituted benzoxazino[4,3-b][1,2,5]thiadiazepinone 6,6-dioxides from polymer-supported Fmoc-Ser(tBu)-OH and Fmoc-Thr(tBu)-OH. After the solid-phase synthesis of N-alkylated-N-sulfonylated intermediates using various 2-nitrobenzenesulfonyl chlorides and bromoketones, the target compounds were obtained via trifluoroacetic acid (TFA)-mediated cleavage from the resin, followed by cyclization of the diazepinone scaffold. Except for the threonine-based intermediates, the inclusion of triethylsilane (TES) in the cleavage cocktail yielded a specific configuration of the newly formed C3 chiral center. The final cyclization resulted in minor or no inversion of the C12a stereocenter configuration.

Keywords: benzoxazinothiadiazepinone; bromoketone; cysteine; morpholine; nitrobenzenesulfonyl chloride; serine; solid-phase synthesis; stereoselective synthesis; thiomorpholine; threonine; triethylsilane.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alkylation
  • Cyclic S-Oxides / chemical synthesis*
  • Cyclization
  • Polymers / chemistry*
  • Small Molecule Libraries / chemical synthesis
  • Solid-Phase Synthesis Techniques
  • Stereoisomerism
  • Structure-Activity Relationship
  • Thiadiazoles / chemical synthesis*

Substances

  • Cyclic S-Oxides
  • Polymers
  • Small Molecule Libraries
  • Thiadiazoles