New lipases by mining of Pleurotus ostreatus genome

PLoS One. 2017 Sep 25;12(9):e0185377. doi: 10.1371/journal.pone.0185377. eCollection 2017.

Abstract

The analysis of Pleurotus ostreatus genome reveals the presence of automatically annotated 53 lipase and 34 carboxylesterase putative coding-genes. Since no biochemical or physiological data are available so far, a functional approach was applied to identify lipases from P. ostreatus. In the tested growth conditions, four lipases were found expressed, with different patterns depending on the used C source. Two of the four identified proteins (PleoLip241 and PleoLip369), expressed in both analysed conditions, were chosen for further studies, such as an in silico analysis and their molecular characterization. To overcome limits linked to native production, a recombinant expression approach in the yeast Pichia pastoris was applied. Different expression levels were obtained: PleoLip241 reached a maximum activity of 4000 U/L, whereas PleoLip369 reached a maximum activity of 700 U/L. Despite their sequence similarity, these enzymes exhibited different substrate specificity and diverse stability at pH, temperature, and presence of metals, detergents and organic solvents. The obtained data allowed classifying PleoLip241 as belonging to the "true lipase" family. Indeed, by phylogenetic analysis the two proteins fall in different clusters. PleoLip241 was used to remove the hydrophobic layer from wool surface in order to improve its dyeability. The encouraging results obtained with lipase treated wool led to forecast PleoLip241 applicability in this field.

MeSH terms

  • Animals
  • Carboxylesterase / chemistry
  • Carboxylesterase / genetics
  • Carboxylesterase / metabolism
  • Catalytic Domain
  • Coloring Agents
  • Data Mining
  • Fungal Proteins / chemistry
  • Fungal Proteins / genetics*
  • Fungal Proteins / metabolism
  • Genome, Fungal*
  • Industrial Microbiology
  • Kinetics
  • Lipase / chemistry
  • Lipase / genetics*
  • Lipase / metabolism
  • Models, Molecular
  • Phylogeny
  • Pleurotus / enzymology*
  • Pleurotus / genetics*
  • Recombinant Proteins / chemistry
  • Recombinant Proteins / genetics
  • Recombinant Proteins / metabolism
  • Substrate Specificity
  • Wool

Substances

  • Coloring Agents
  • Fungal Proteins
  • Recombinant Proteins
  • Carboxylesterase
  • Lipase

Grants and funding

V. T. and L. G. acknowledge Università degli Studi di Napoli Federico II for doctoral fellowships.