Asymmetric synthesis of tetrahydroquinoline-type ecdysone agonists and QSAR for their binding affinity against Aedes albopictus ecdysone receptors

Pest Manag Sci. 2019 Jan;75(1):115-124. doi: 10.1002/ps.5160. Epub 2018 Oct 9.

Abstract

Background: Tetrahydroquinolines (THQs) are a class of non-steroidal ecdysone agonists that specifically bind to mosquito ecdysone receptors (EcR). The THQ scaffold contains two chiral centers at the C-2 and C-4 positions, resulting in four stereoisomers. We have previously shown that the (2R,4S)-isomers are the most biologically active; however, the lack of a practical synthetic method for these isomers has hampered further structure-activity studies.

Results: In this study, a chiral phosphoric acid-catalyzed Povarov reaction was employed to develop a facile asymmetric synthesis of THQs with a (2R,4S)-configuration, which allowed the preparation of a 40-compound library of enantiopure THQs. Evaluation of their binding affinity against Aedes albopictus EcR, followed by quantitative structure-activity relationship (QSAR) analyses, uncovered the physicochemical properties of THQs that are important for the ligand-receptor interaction. The most potent THQ derivative was twofold more active than the molting hormone, 20-hydroxyecdysone.

Conclusion: The QSAR results provide valuable information for the rational design of novel mosquito-specific ecdysone agonists. © 2018 Society of Chemical Industry.

Keywords: QSAR; asymmetric synthesis; ecdysone; mosquito; tetrahydroquinoline.

MeSH terms

  • Aedes / metabolism*
  • Animals
  • Ecdysone / agonists*
  • Insect Proteins / metabolism*
  • Protein Binding
  • Quantitative Structure-Activity Relationship
  • Quinolines / chemical synthesis*
  • Receptors, Steroid / metabolism*

Substances

  • Insect Proteins
  • Quinolines
  • Receptors, Steroid
  • ecdysone receptor
  • Ecdysone