A novel interleukin-13 receptor alpha 2-targeted hybrid peptide for effective glioblastoma therapy

Chem Biol Drug Des. 2019 Jul;94(1):1402-1413. doi: 10.1111/cbdd.13517. Epub 2019 Apr 22.

Abstract

We previously designed and reported a novel class of drugs, namely hybrid peptides, which are chemically synthesized and composed of a targeted binding peptide and a lytic-type peptide containing cationic amino acid residues that cause cancer cell death. In the present study, we screened for peptides that bind to interleukin-13 receptor alpha 2 (IL-13Rα2) by using a T7 random peptide phage display library system and isolated several positive phage clones. The A2b11 peptide, which was one of the positive clones, was shown to bind to IL-13Rα2 protein by Biacore analysis and a binding assay using glioblastoma (GB) cell lines. This peptide was linked with a lytic peptide containing a linker sequence to form the IL-13Rα2-lytic hybrid peptide. The IL-13Rα2-lytic hybrid peptide showed cytotoxic activity against GB cell lines in vitro. The IL-13Rα2-lytic hybrid peptide also affected Akt and Erk1/2 activation following treatment with interleukin-13 and induced rapid ATP dynamics in GB cells. Anti-tumor activity of the IL-13Rα2-lytic hybrid peptide was observed in vivo after intratumoral injection in a mouse xenograft model of human GB cells. These results suggest that the IL-13Rα2-lytic hybrid peptide might be a potent therapeutic option for patients with GB.

Keywords: IL-13Rα2; T7 phage display; glioblastoma; hybrid peptide; molecularly targeted therapy.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Antineoplastic Agents / chemistry*
  • Antineoplastic Agents / pharmacology
  • Antineoplastic Agents / therapeutic use
  • Cell Line, Tumor
  • Cell Survival / drug effects
  • Drug Design
  • Female
  • Glioblastoma / drug therapy
  • Glioblastoma / pathology
  • Humans
  • Interleukin-13 Receptor alpha2 Subunit / antagonists & inhibitors*
  • Interleukin-13 Receptor alpha2 Subunit / genetics
  • Interleukin-13 Receptor alpha2 Subunit / metabolism
  • Mice
  • Mice, Nude
  • Mitogen-Activated Protein Kinase 3 / metabolism
  • Peptide Library
  • Peptides / chemistry*
  • Peptides / metabolism
  • Peptides / pharmacology
  • Peptides / therapeutic use
  • Proto-Oncogene Proteins c-akt / metabolism
  • Recombinant Proteins / biosynthesis
  • Recombinant Proteins / chemistry
  • Signal Transduction / drug effects
  • Xenograft Model Antitumor Assays

Substances

  • Antineoplastic Agents
  • Interleukin-13 Receptor alpha2 Subunit
  • Peptide Library
  • Peptides
  • Recombinant Proteins
  • Proto-Oncogene Proteins c-akt
  • Mitogen-Activated Protein Kinase 3