High-Throughput LC-MS/MS Method for Chiral Amino Acid Analysis Without Derivatization

Methods Mol Biol. 2019:2030:253-261. doi: 10.1007/978-1-4939-9639-1_19.

Abstract

D-Amino acids have recently attracted much attention in various research fields including medical, clinical, and food industry due to their important biological functions that differ from L-amino acid. Most chiral amino acid separation techniques require complicated derivatization procedures in order to achieve the desirable chromatographic behavior and detectability. This chapter describes a highly sensitive analytical method for the enantioseparation of chiral amino acids without any derivatization process using liquid chromatography-tandem mass spectrometry (LC-MS/MS). The method allows the simultaneous analysis of 18 D-amino acids with high sensitivity and reproducibility. Additionally, this chapter also focuses on the application of the method to real samples for the quantification of targeted amino acids.

Keywords: Chiral; D-Amino acid; Enantioseparation; LC-MS/MS; Quantitative analysis; Underivatized.

Publication types

  • Validation Study

MeSH terms

  • Amino Acids / analysis*
  • Amino Acids / chemistry
  • Chromatography, High Pressure Liquid / instrumentation
  • Chromatography, High Pressure Liquid / methods
  • High-Throughput Screening Assays / instrumentation
  • High-Throughput Screening Assays / methods*
  • Reproducibility of Results
  • Sensitivity and Specificity
  • Stereoisomerism
  • Tandem Mass Spectrometry / instrumentation
  • Tandem Mass Spectrometry / methods*

Substances

  • Amino Acids