Spatio-temporal patterns of air pollution in China from 2015 to 2018 and implications for health risks

Abstract

China has been seriously affected by particulate matter (PM) and gaseous pollutants in the atmosphere. In this study, we systematically analyse the spatio-temporal patterns of PM_2.5, PM₁₀, SO₂, CO, NO₂, and O₃ and the associated health risks, using data collected from 1498 national air quality monitoring sites. An analysis of the averaged data from all the sites indicated that, from 2015 to 2018, annual mean concentrations of PM_2.5, PM₁₀, SO₂ and CO declined by 3.2 μg m^-3, 3.7 μg m^-3, 3.9 μg m^-3, and 0.1 mg m^-3, respectively. In contrast, those of NO₂ and O₃ increased at rates of 0.4 and 3.1 μg m^-3, respectively. Except for O₃, the annual mean concentrations of all pollutants were generally the highest in North China and lowest in the Tibetan Plateau. The concentrations were generally higher in the north of the country than in the south. In all regions of China, the pollutant concentrations were the highest in winter and lowest in summer, except for O₃, which showed an opposite seasonal pattern. Overall, the seasonal mean concentrations of all the pollutants (except for O₃) significantly decreased between the same seasons in 2018 and 2015, whereas the seasonal mean O₃ concentrations generally significantly increased, and/or remained at stable levels in all four seasons except for winter. Diurnal variations of all pollutants (except for O₃) exhibited a bimodal pattern with peaks between 8:00 and 11:00 a.m. and 9:00 and 12:00 p.m., whereas O₃ exhibited a unimodal pattern with maximum values between 5:00 and 7:00 p.m. No significant differences in the daily mean concentrations of all pollutants were found between weekdays and weekends in all regions, except for PM_2.5 and PM₁₀ in Northeast China. In Northwest China and Southeast China, PM_2.5 showed stronger correlations with NO₂ relative to SO₂, suggesting that NO_x emission control may be more effective than SO₂ emission control for alleviating PM_2.5 formation. Compared with 2015, the total PM_2.5-attributable mortality, number of respiratory and cardiovascular diseases, and incidence of chronic bronchitis decreased overall by 23.4%-26.9% in 2018. In contrast, for O₃-attributable deaths, there was an increase of 18.9%. Our study not only improves the understanding of the spatial and temporal patterns of air pollutants in China, but also highlights that synchronous control of PM_2.5 and O₃ pollution should be implemented to achieve dual benefits in protecting human health.

Keywords: Air pollution; China; Emission control; Human health; Ozone; PM(2.5).