Tumor-targeted delivery of silibinin and IPI-549 synergistically inhibit breast cancer by remodeling the microenvironment

Int J Pharm. 2020 May 15;581:119239. doi: 10.1016/j.ijpharm.2020.119239. Epub 2020 Mar 16.

Abstract

We induced changes in the tumor microenvironment (TME) through the synergistic actions of two drugs used in breast cancer therapy. The anti-fibrotic drug silibinin (SLB) targets tumor-associated fibroblasts and exerts immune-mediated anti-cancer effects. IPI-549, an efficient and highly selective phosphoinositide-3-kinase-gamma (PI3Kγ) inhibitor, was applied to alter the balance of immunosuppressive cells by inhibiting PI3Kγ molecules; it also promotes anti-tumor immunity. We developed nanoparticle formulations to encapsulate both drugs into the targeting carrier aminoethyl anisamide-polyethylene glycol-polycaprolactone (AEAA-PEG-PCL) respectively. The drugs were intravenously delivered in mice and resulted in an increase in anti-tumor efficacy and apoptotic tumor tissue compared with either IPI-549 or SLB alone in 4T1 breast cancer cell-derived tumors. Furthermore, a significant reduction in regulatory T (Treg) cells and myeloid suppressor cells (MDSCs) was observed. A normalized TME structure was also observed, including angiogenesis suppression, antifibrotic effects and the inhibition of collagen formation in the tumor tissue, significantly enhancing the anti-tumor effects. In summary, this combination strategy may offer an alternative treatment for breast cancer.

Keywords: Breast cancer; IPI-549; Nanoparticle; Silibinin; Tumor microenvironment.

MeSH terms

  • Administration, Intravenous
  • Animals
  • Antineoplastic Agents, Phytogenic / administration & dosage
  • Antineoplastic Agents, Phytogenic / pharmacokinetics
  • Antineoplastic Combined Chemotherapy Protocols / administration & dosage*
  • Antineoplastic Combined Chemotherapy Protocols / pharmacokinetics
  • Benzamides / chemistry
  • Breast Neoplasms / drug therapy*
  • Breast Neoplasms / pathology
  • Cancer-Associated Fibroblasts
  • Cell Line, Tumor / transplantation
  • Disease Models, Animal
  • Drug Carriers / chemistry*
  • Drug Evaluation, Preclinical
  • Drug Screening Assays, Antitumor
  • Drug Synergism
  • Female
  • Humans
  • Isoquinolines / administration & dosage*
  • Isoquinolines / pharmacokinetics
  • Mice
  • Nanoparticles / chemistry
  • Polyesters / chemistry
  • Polyethylene Glycols / chemistry
  • Protein Kinase Inhibitors / administration & dosage
  • Protein Kinase Inhibitors / pharmacokinetics
  • Pyrazoles / administration & dosage*
  • Pyrazoles / pharmacokinetics
  • Pyrimidines / administration & dosage*
  • Pyrimidines / pharmacokinetics
  • Silybin / administration & dosage*
  • Silybin / pharmacokinetics
  • Tumor Microenvironment / drug effects

Substances

  • Antineoplastic Agents, Phytogenic
  • Benzamides
  • Drug Carriers
  • Isoquinolines
  • Polyesters
  • Protein Kinase Inhibitors
  • Pyrazoles
  • Pyrimidines
  • polycaprolactone-g-polyethylene glycol
  • Polyethylene Glycols
  • Silybin
  • N-(2-aminoethyl)-2-anisamide
  • IPI-549