Antineoplastic drug-loaded polymer-modified magnetite nanoparticles: Comparative analysis of EPR-mediated drug delivery

Cell Biol Int. 2020 Oct;44(10):2042-2052. doi: 10.1002/cbin.11413. Epub 2020 Jul 16.

Abstract

This study aimed to design and evaluate enhanced permeation and retention (EPR)-mediated anticancer effect of polymer-modified and drug-loaded magnetite nanocomposites. The preformulated bare (10 nm), chitosan-superparamagnetic iron oxide (SPIO; 69 nm), heparin-SPIO (42 nm), and (3-aminopropyl)triethoxysilane-polyethylene glycol-SPIO (17 nm) nanocomposites were utilized to evaluate the EPR-mediated localized cancer targeting and retention of doxorubicin (DOX) and paclitaxel (PTX) in human ovarian cancer cell lines, A2780 and OVCAR-3 in vitro and in the tumor-baring Balb/c mice in vivo. Fluorescence microscopy showed that DOX- and PTX-loaded SPIO nanoparticles caused long-term accumulation and cytoplasmic retention in A2780 and OVCAR-3 cells, as compared to free drugs in vitro. In vivo antiproliferative effect of present formulations on immunodeficient female Balb/c mice showed a tremendous amount of ovarian tumor shrinkage within 6 weeks. The present nanocomposite systems of targeted drug delivery proved to be efficient drug carrier with sustained drug release and long-term retention with enhanced cytotoxic properties in vitro and in vivo.

Keywords: Balb/c mice; biodegradable nanocomposites; enhanced permeation; sustained release; tumor volume.

MeSH terms

  • Animals
  • Antineoplastic Agents / pharmacology*
  • Cell Line, Tumor
  • Chitosan / chemistry
  • Doxorubicin / pharmacology*
  • Drug Carriers / administration & dosage*
  • Female
  • Humans
  • Magnetite Nanoparticles / administration & dosage*
  • Mice, Inbred BALB C
  • Mice, SCID
  • Ovarian Neoplasms / drug therapy*
  • Polyethylene Glycols / chemistry
  • Propylamines / chemistry
  • Silanes / chemistry

Substances

  • Antineoplastic Agents
  • Drug Carriers
  • Magnetite Nanoparticles
  • Propylamines
  • Silanes
  • Polyethylene Glycols
  • Doxorubicin
  • Chitosan
  • amino-propyl-triethoxysilane