Hydrogen Production through Catalytic Water Splitting Using Liquid-Phase Plasma over Bismuth Ferrite Catalyst

Int J Mol Sci. 2021 Dec 18;22(24):13591. doi: 10.3390/ijms222413591.

Abstract

This study examined the H2 production characteristics from a decomposition reaction using liquid-phase plasma with a bismuth ferrite catalyst. The catalyst was prepared using a sol-gel reaction method. The physicochemical and optical properties of bismuth ferrite were analyzed. H2 production was carried out from a distilled water and aqueous methanol solution by direct irradiation via liquid-phase plasma. The catalyst absorbed visible-light over 610 nm. The measured bandgap of the bismuth ferrite was approximately 2.0 eV. The liquid-phase plasma emitted UV and visible-light simultaneously according to optical emission spectrometry. Bismuth ferrite induced a higher H2 production rate than the TiO2 photocatalyst because it responds to both UV and visible light generated from the liquid-phase plasma.

Keywords: H2 production; bismuth ferrite; liquid-phase plasma; optical emission; water splitting.

MeSH terms

  • Bismuth / chemistry*
  • Catalysis
  • Ferric Compounds / chemistry*
  • Hydrogen / chemistry*
  • Phase Transition
  • Plasma Gases / chemistry
  • Water / chemistry*

Substances

  • Ferric Compounds
  • Plasma Gases
  • Water
  • ferrite
  • Hydrogen
  • Bismuth