Examination of the Novel Sigma-1 Receptor Antagonist, SI 1/28, for Antinociceptive and Anti-allodynic Efficacy against Multiple Types of Nociception with Fewer Liabilities of Use

Int J Mol Sci. 2022 Jan 6;23(2):615. doi: 10.3390/ijms23020615.

Abstract

Neuropathic pain is a significant problem with few effective treatments lacking adverse effects. The sigma-1 receptor (S1R) is a potential therapeutic target for neuropathic pain, as antagonists for this receptor effectively ameliorate pain in both preclinical and clinical studies. The current research examines the antinociceptive and anti-allodynic efficacy of SI 1/28, a recently reported benzylpiperazine derivative and analog of the S1R antagonist SI 1/13, that was 423-fold more selective for S1R over the sigma-2 receptor (S2R). In addition, possible liabilities of respiration, sedation, and drug reinforcement caused by SI 1/28 have been evaluated. Inflammatory and chemical nociception, chronic nerve constriction injury (CCI) induced mechanical allodynia, and adverse effects of sedation in a rotarod assay, conditioned place preference (CPP), and changes in breath rate and locomotor activity were assessed after i.p. administration of SI 1/28. Pretreatment with SI 1/28 produced dose-dependent antinociception in the formalin test, with an ED50 (and 95% C.I.) value of 13.2 (7.42-28.3) mg/kg, i.p. Likewise, SI 1/28 produced dose-dependent antinociception against visceral nociception and anti-allodynia against CCI-induced neuropathic pain. SI 1/28 demonstrated no impairment of locomotor activity, conditioned place preference, or respiratory depression. In summary, SI 1/28 proved efficacious in the treatment of acute inflammatory pain and chronic neuropathy without liabilities at therapeutic doses, supporting the development of S1R antagonists as therapeutics for chronic pain.

Keywords: allodynia; analgesia; antagonist; neuropathic pain; sedation; sigma; sigma-1 receptor.

MeSH terms

  • Analgesics / administration & dosage
  • Analgesics / pharmacology
  • Analgesics / therapeutic use*
  • Animals
  • Disease Models, Animal
  • Hyperalgesia / complications
  • Hyperalgesia / drug therapy*
  • Inflammation / complications
  • Inflammation / pathology
  • Male
  • Mice
  • Mice, Inbred C57BL
  • Nociception*
  • Receptors, sigma / antagonists & inhibitors*
  • Receptors, sigma / metabolism
  • Sigma-1 Receptor
  • Time Factors
  • Viscera / pathology

Substances

  • Analgesics
  • Receptors, sigma