Synthesis, Processing and the Effect of Thermal Treatment on the Solubility, Antioxidant Potential and Cytocompatibility of Y2O3 and CeO2 doped SiO2-SrO-Na2O Glass-Ceramics

J Biomater Appl. 2022 Jul;37(1):102-117. doi: 10.1177/08853282221078448. Epub 2022 Apr 20.

Abstract

Thermal treatment of a 0.52SiO2-0.24SrO-0.24-xNa2O-xMO glass-ceramic series (where x = 0.08 and MO = Y2O3 or CeO2) was conducted in order to synthesize yttrium (Y3+) and cerium (Ce3+) crystalline species that may act as radical oxygen specie (ROS) scavengers. The prominent phase for the Control is a sodium-strontium-silicate while the experimental glass-ceramics (HY, YCe, and HCe) present sodium-Y/Ce-silicate and oxide phases. Disk shrinkage during thermal processing ranges from 1-7% for Control, HY, YCe, and HCe in both diameter and thickness. Solubility studies determined that the release of Si4+ and Na+ are greatest from the Control disks which peaks at 1550 µg/mL. Release from the Y3+ and Ce3+ glass-ceramics reached 320 µg/mL for Si4+ and 630 µg/mL for Na+. The range of antioxidant capacity (ABTS assay) for all samples was 0.31-3.9 mMTE. No significant reduction in MC 3T3 Osteoblast cell viability was observed for any composition tested.

Keywords: antioxidant capacity; bioactive glass; bioceramic; cerium; nerve; yttrium.

MeSH terms

  • Antioxidants*
  • Ceramics / chemistry
  • Glass / chemistry
  • Oxides / chemistry
  • Silicates
  • Silicon Dioxide* / chemistry
  • Sodium
  • Sodium Compounds
  • Solubility
  • Yttrium

Substances

  • Antioxidants
  • Oxides
  • Silicates
  • Sodium Compounds
  • sodium oxide
  • Yttrium
  • Silicon Dioxide
  • Sodium
  • yttria