Desalination by solar steam generation (SSG) system is a green technology to produce pure water, which can address the issue of water scarcity. A novel photothermal material for the SSG system was fabricated by immersing bacterial cellulose (BC) sequentially into tannic acid (TA) and iron(iii) (Fe3+) solutions. Surface analysis of the resulting BC-TA-Fe3+ (BTF) material showed that coordination nanocomplexes between Fe3+ and hydroxyl groups of TA were formed on the surface of cellulose nanofibers. BTF material exhibited high sunlight absorption (∼95%), hydrophilic, self-cleaning properties, and excellent structural stability. SSG systems based on BTF had an evaporation efficiency of 91% and an evaporation rate of 1.56 kg m-2 h-1 under 1 sun illumination. Then, an efficient desalination device based on the larger-scale BTF material was fabricated to produce freshwater, the amount of freshwater per day was 5.6 kg m-2 on a sunny day. BTF material, thus, showed great potential in seawater desalination applications along with simple, versatile, scalable, and affordable fabrication methods.
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