Co-Benefits of Pollutant Removal, Water, and Heat Recovery from Flue Gas through Phase Transition Enhanced by Corona Discharge

Environ Sci Technol. 2022 Jun 21;56(12):8844-8853. doi: 10.1021/acs.est.2c00917. Epub 2022 May 27.

Abstract

Pollutant removal and resource recovery from high-humidity flue gas after desulfurization in a thermal power plant are crucial for improving air quality and saving energy. This study developed a flue gas treatment method involving phase transition enhanced by corona discharge based on laboratory research and established a field-scale unit for demonstration. The results indicate that an adequate increase in size will improve the ease of particle capture. A wet electrostatic precipitator is applied before the condensing heat exchangers to enhance the particle growth and capture processes. This results in an increase of 58% in the particle median diameter in the heat exchanger and an emission concentration below 1 mg/m3. Other pollutants, such as SO3 and Hg, can also be removed with emission concentrations of 0.13 mg/m3 and 1.10 μg/m3, respectively. Under the condensation enhancement of the method, it is possible to recover up to 3.26 t/h of water from 200 000 m3/h saturated flue gas (323 K), and the quality of the recovered water meets the standards stipulated in China. Additionally, charge-induced condensation is shown to improve heat recovery, resulting in the recovery of more than 43.34 kJ/h·m3 of heat from the flue gas. This method is expected to save 2628 t of standard coal and reduce carbon dioxide emission by 2% annually, contributing to environmental protection and global-warming mitigation.

Keywords: carbon reduction; condensation; corona discharge; pollutant control; waste heat recovery; water recovery.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Air Pollutants* / analysis
  • Coal
  • Environmental Monitoring / methods
  • Environmental Pollutants*
  • Hot Temperature
  • Power Plants
  • Water

Substances

  • Air Pollutants
  • Coal
  • Environmental Pollutants
  • Water